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Highly efficient halide-tolerant dioxygen photoreduction in a metal-organic framework.
Dioxygen photoreduction is of great importance for the production of renewable fuels and chemicals from solar energy. However, most of the state-of-the-art systems exhibit severe deactivation of the photocatalyst by a variety of chemical and physical factors. Here we report the use of a rigid metal-organic framework (MOF) with two open metal sites to achieve effective halide-tolerant dioxygen photoreduction in water. Under the irradiation of visible light, dioxygen was efficiently reduced to H(2)O(2) by a new Ru(II)-containing MOF. The selectivity of dioxygen reduction is remarkably high: >98.7% of H(2)O(2) can be produced with >99.9% selectivity. Dioxygen photoreduction is highly effective in a broader wavelength range of visible light (450-700 nm) compared to previous reports. We also show that the Ru sites in the MOF have catalytic activity for dioxygen photoreduction, with almost 100% conversion to H(2)O(2) after several turnovers of dioxygen photoreduction. These results demonstrate the importance of the structural features of the photocatalytic material, providing a promising way to develop new photosynthetic catalysts for efficient solar energy conversion.Q:
Why does LyX disable hotkeys on Mac OSX?
I am writing a thesis in LyX and occasionally I have to click on menu bar buttons in order to make the main menu popup. I am on OSX 10.7.3 and don't know if this is the issue, but all the while the hotkeys are disabled on the Mac.
I know this because the hotkey popup says so. 01e38acffe
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As experts worldwide have warned that there is no proven coronavirus vaccine, the British government is currently not offering immunizations to the general public, but it does recommend the Public Health England's COVID-19 vaccine research program -- a free, voluntary program.
And amid the European Union (EU) funding crisis that has left countries without money and vaccine research programs underfunded, the UK is offering free immunization to any workers who are not already covered under a workers' compensation program.
This program, which will last for eight weeks, was announced on Friday by British Prime Minister Boris Johnson's office.
"We have therefore launched a targeted Public Health campaign for those employees who do not already benefit from employer-funded workplace immunization programmes," the office said in a statement.
In a statement, Public Health England said, "They should consider asking their employer to participate in the free vaccination campaign. However, Public Health England does not recommend that we recommend a vaccination to the public at this time.”
PATIENT IS MY 'BELLYACHING' NEW FRIEND: 'I AM NOT PRACTICING MY HAND SIGNALS FOR HIM'
Johnson told Parliament on Monday that scientists are working with pharmaceutical companies to create a COVID-19 vaccine, but that it would take a year to manufacture one. He has stressed that there is no cure for COVID-19 and therefore prevention is key.
However, the EU vaccine research program is currently underfunded and Germany, France and other countries within the bloc have complained that their research programs have been underfunded in recent years.
COVID-19 has already claimed the lives of hundreds of thousands of people in the U.S. and around the world and has affected more than 28 million others.
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The U.S. has been the hardest hit by the pandemic so far, but there are still more than 1,500 U.S. deaths attributed to COVID-19./*
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